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X XHBX #3ؑ|=sǜ{ӌӄY.%eeBaԔ36c/ aL#T2/4v̨vT+QQڵFkM톂TòJi<'8WXs$*$Ӵ>8W8֎64\mL,% TDأ ~[ 2n}1a0o2bb]1n*e%@gKNvpOhں[dnؽvΝVٰg|pEu};X=>k_\+/>kN]}KA./G#&UB`?- u_i!7)B'M;v{T/mt's`iho<3P!14f}4"}O"Q<椆UJeW C) )!_TN}{D,MbI%f|T-i-Pjl <8;2Xq+4~֥) I$J0 UBEl~O~-LBGȆ"!|H:Gqoo)k>4N<_,&dMɌOfN_rSSiw}M0 6U؝%]rt6$(hR~59塦W&G @뤘\$ JU|T-#-<~s*!EvF;icCa @:vo9*mX euZpw߿j^ej 0.[et,;>7.& jDEeX($Xܹb:V'ʓڧo84 8-O?7Z c*bo.1q< `Pեl&&3[GG|3,FT9Qq..+:ά}}r'2 sRN_D endstream endobj 42 0 obj <>stream 2022-05-27T14:23:46+08:00 2022-05-27T14:23:40+08:00 2022-05-27T14:23:46+08:00 Acrobat PDFMaker 11 Word 版 uuid:202d69de-9f12-44e3-a8ab-641a19e198be uuid:7c7bf6e0-4dca-42f3-b77f-d3b11b6114e4 8 application/pdf 原位制备混二甲苯磺酸及其催化合成TMPTMA 以工业生产二甲苯的精馏剩余物(主要成分为邻、间、对–二甲苯)和98%硫酸反应制备得到混二甲苯磺酸作为催化剂,以三羟甲基丙烷(TMP)、甲基丙烯酸(MA)为原料,采用共沸酯化法合成三羟甲基丙烷三甲基丙烯酸酯(TMPTMA)。研究了催化剂用量、外加热源温度、反应时间对酯化过程的影响,结果表明最适于本反应的条件为催化剂质量为TMP与MA质量之和的5%、外加热源温度为130℃、反应时间为8小时,在此条件下原料TMP与MA的转化率、反应酯化率均在98%以上。分别采用GC和GC-MS对产品进行了纯度检测和定性分析。通过对比,发现自制混二甲苯磺酸催化效果明显优于98%硫酸、与工业对甲苯磺酸具有几乎相同的催化性能。为解决工业生产二甲苯的精馏剩余物(主要成分为邻、间、对–二甲苯)提供了一种资源化利用思路。 邵玉田,关情,丁春燕,程志远,程林轩 Adobe PDF Library 11.0 二甲苯,三羟甲基丙烷三甲基丙烯酸酯(TMPTMA),精馏剩余物,催化剂,共沸酯化法 D:20220527062326 以工ä¸ıçfl�产亄çfl²è‰¯çı—精馑囩低盩(主覆拒勃为釻㕆銴㕆对â•fi亄çfl²è‰¯)噄98%硫閸呓åºfl勶å¤⁄徊勰混亄çfl²è‰¯ç£ºé–¸ä½œä¸ºå‡¬å„Œå›‡ï¼„以丛ç¾�çfl²å�ºä¸Žç…·(TMP)㕆çfl²å�ºä¸Žç…¯é–¸(MA)为å”�挎$é⁄⁄çfl¨å–±æ²¸é–¯å„Œæ³Łå’‹æ‹’丛ç¾�çfl²å�ºä¸Žç…·ä¸›çfl²å�ºä¸Žç…¯é–¸é–¯(TMPTMA)㕇ç€fl究亃凬儌囇çfl¨é⁄‘㕆夌å−€ç…�溒温度㕆呓åºfl抶銴对閯儌è¿⁄稉çı—å½±åfi“$ç»fi果表柔朕镇五本呓åºflçı—暡件为凬儌囇质é⁄‘为TMP且MAè´¨é⁄‘义噄çı—5%㕆夌å−€ç…�溒温度为130◅㕆呓åºfl抶銴为8少抶$在æ�¤æš¡ä»¶ä¸‰å”�挎TMP且MAçı—转儌ç”⁄㕆呓åºfl閯儌ç”⁄åš⁄在98%以ä¸−㕇勃勫é⁄⁄çfl¨GC噄GC-MS对产åfi†è¿łè¡„亃纯度棕浉噄å®ı敧勃枒㕇é•ıè¿⁄对æ¯fl$呂田è⁄ªå‹¶æ··äº„çfl²è‰¯ç£ºé–¸å‡¬å„ŒæŁ‹æžœæŸ”柾伟五98%硫閸㕆且工ä¸ı对çfl²è‰¯ç£ºé–¸å–·æœ›å⁄€ä¹”çł¸å’„çı—凬儌敧腽㕇为解僳工ä¸ıçfl�产亄çfl²è‰¯çı—精馑囩低盩(主覆拒勃为釻㕆銴㕆对â•fi亄çfl²è‰¯)æ‘’ä¾łäºƒä¸•ç§“èµ—æº’å„Œå‹©çfl¨æ•šè·¯ã•‡ endstream endobj 43 0 obj <>stream h24S0Pw/+Q0L)620)BH(e <#0/V? 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