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FF๳؉{>{ ZI:6CmuUԕǙ]XF=ל*xOPe1CczS aa&6""mgDY  G'N?ݞ<*f_Aw5or質3b:Q qA//KdDG6O$ gr,&v"8>^llcceKӜ,#of5dkc6Lc q \ -dn=La@l'e&K)3j AnxF#Qd%^Ak\!Ib'?(-9aRv2x% jPj@)n<-RJ%Pj=4"XRb͡**'{ݬ?o Og:*QNSr,Lm=2Gre㉼\v^.9E.5jû7LVK,j5~)HW/?nrkGZ𔱘̕#)"]kR*R?Ȓ endstream endobj 45 0 obj <>stream 2021-05-28T13:04:22+08:00 2021-05-28T13:04:17+08:00 2021-05-28T13:04:22+08:00 Acrobat PDFMaker 11 Word 版 uuid:cf529072-09ac-497c-868b-3d0cdc9da35e uuid:0e2d285d-796e-4687-87de-0b0edfff5bd2 341 application/pdf 电化学条件下磺酰肼与烯醇硅醚自由基偶联反应合成β-羰基砜化合物 β-羰基砜是一类重要的有机合成砌块,合成该类化合物一直是研究热点。本文以四丁基碘化铵为媒介,在电化学条件下实现烯醇硅醚与各种取代的磺酰肼发生自由基磺酰化反应,经自由基加成和氧化,在最优条件下以55%~76%的收率合成了8种具有不同取代基的β-羰基砜类化合物。采用核磁共振和质谱等手段对产物结构进行表征,并提出了可能的反应机理。 王杨丽,周烨,曾东文,何永辉 Adobe PDF Library 11.0 β-羰基砜,电催化,自由基偶联反应 D:20210528050407 β-ç¾°å�ºç€œæŸ¯ä¸•ç±»é⁄“覆çı—æœ›æœºå’‹æ‹’ç€„åšŠï¼„å’‹æ‹’è¯¥ç±»å„Œå’‹ç›©ä¸•çł´æŸ¯ç€fl究ç…�燹㕇本æŒ⁄ä»¥åłłä¸†å�ºç¢Ÿå„Œéfiµä¸ºåª™ä»‰ï¼„在çflµå„Œå�¦æš¡ä»¶ä¸‰å®žç”°ç…¯éƒ⁄ç¡–éƒı且咗秓呌代çı—磺閰臼呂çfl�è⁄ªçfl±å�ºç£ºé–°å„Œå‘“åºfl$绑è⁄ªçfl±å�ºå−€æ‹’噄氧儌$在朕伟暡件三以55%~76%çı—æfl¶ç”⁄咋拒亃8秓喷望专咄呌代å�ºçı—β-ç¾°å�ºç€œç±»å„Œå’‹ç›©ã•‡é⁄⁄çfl¨æ€¸ç£†å–±æ„¯å™„质谱ç�›æ›‰æ®µå¯¹äº§ç›©ç»fiæž—è¿łè¡„è¡¨å¾†ï¼„å¹¶æ‘’å⁄ºäºƒå‘¯è…½çı—å‘“åºfl机璃㕇 endstream endobj 46 0 obj <>stream h2P0Pw/+Q0L)620)I 14SFDT$! endstream endobj 47 0 obj <>stream h2T0Pw,-/;=?OHF7ES7?{ (O)MN-pLOJUpqSL*J,T043/-JNd9PAiRVjr j'l,kIL H ":X,(ӏK~HUYۂL:~On1M,6嫟U$yc4JMŢqG+P~b{Y~|!,g=.k5aORyHHbSw" I 'G^@c% =e0BU:s3ղTv,*s UւpMu /KLhdXT ,L1LoyQf>yʒ/k ~t6&M̒T`"??>QT Ѵ0 endstream endobj 48 0 obj <>/Filter/FlateDecode/ID[<1A01CE6995E2AE42BF6775B1E189AC11>]/Info 199 0 R/Length 223/Root 201 0 R/Size 200/Type/XRef/W[1 3 1]>>stream hbb&F  L@ )n"YH0"^H``fm6`qbj2`G- 6s}\ ,1' Dj0Hp-G`5dV w!c:3µ`LNA*"TZLCl;b[;ơD2?FaG+?Gl^,_wUVn`4Cm 5k& endstream endobj startxref 116 %%EOF